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    ARTICLE

    Computer Modeling of Ionic Conductivity in Low Temperature Doped Ceria Solid Electrolytes

    Shu-Feng Lee1, Che-Wun Hong1,2

    CMC-Computers, Materials & Continua, Vol.12, No.3, pp. 223-236, 2009, DOI:10.3970/cmc.2009.012.223

    Abstract Solid oxides, such as ceria (CeO2) doped with cations of lower valance, are potential electrolytes for future solid oxide fuel cells. This is due to the theoretically high ionic conductivity at low operation temperature. This paper investigates the feasibility of two potential electrolytes which are samarium-doped ceria (SDC) and gadolinium-doped ceria (GDC) to replace the traditional yttria-stablized zirconia (YSZ). Molecular simulation techniques were employed to study the influence of different dopant concentrations at different operation temperatures on the ionic conductivity from the atomistic perspective. Simulation results show that the optimized ionic conductivity occurs at 11.11mol% concentration More >

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