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  • Open Access

    ARTICLE

    Thermosensitive and Wound-Healing Gelatin-Alginate Biopolymer Hydrogels Modified with Humic Acids

    Denis Miroshnichenko1, Vladimir Lebedev2, Katerina Lebedeva2, Аnna Cherkashina2, Sergey Petrushenko3,4,*, Olena Bogoyavlenska1, Аnzhela Olkhovska5, Ihor Hrubnyk6, Liudmyla Maloshtan6, Natalja Klochko7

    Journal of Renewable Materials, Vol.12, No.10, pp. 1691-1713, 2024, DOI:10.32604/jrm.2024.054769 - 23 October 2024

    Abstract The main goal of the article is the creation and study of thermosensitive and wound-healing gelatin-alginate biopolymer hydrogels modified with humic acids. Their rheological properties, swelling and contraction behavior were experimentally investigated, elucidated using Fourier transform infrared spectroscopy and used to achieve the physiological melting point, which is necessary for successful drug delivery. It has been shown that in the gelatin-alginate-humic acid biopolymer hydrogels systems, it is possible to obtain a gel-sol transition temperature close to the physiological temperature of 37°C, which is important for drug delivery in the treatment of wounds. By changing the… More >

  • Open Access

    ARTICLE

    Advanced Nanocomposite Arabic Gum Polyacrylic Acid Hydrogels for Flexible Supercapacitors

    Borhan Albiss*, Asala Saleh

    Journal of Renewable Materials, Vol.12, No.7, pp. 1219-1236, 2024, DOI:10.32604/jrm.2024.050685 - 21 August 2024

    Abstract In this work, the fabrication and characterization of the nanocomposite hydrogel, as a solid electrode in electrochemical cell and gel electrolyte material using Indium titanium oxide/polyethylene terephthalate (ITO/PET) flexible substrate for double-layer supercapacitors have been reported. The nanocomposite hydrogel composed of Arabic gum (AG), Acrylic acid (AA), reduced graphene oxide (RGO), and silver nanoparticles (AgNPs) was fabricated via a physical cross-linked polymerization reaction, in which the ascorbic acid was used as a reducing agent to generate AgNPs and to convert Graphene oxide (GO) to RGO during the polymerization reaction. The morphology and structural characteristics of… More > Graphic Abstract

    Advanced Nanocomposite Arabic Gum Polyacrylic Acid Hydrogels for Flexible Supercapacitors

  • Open Access

    ARTICLE

    Effect of Bio-Based Organic‒Inorganic Hybrid Hydrogels on Fire Prevention of Spontaneous Combustion of Coals

    Hu Shi, Wei Cai, Xin Wang*, Lei Song, Yuan Hu*

    Journal of Renewable Materials, Vol.11, No.12, pp. 3991-4006, 2023, DOI:10.32604/jrm.2023.029888 - 10 November 2023

    Abstract To solve the fire accidents caused by coal combustion, this work prepared four hybrid hydrogel materials using bio-based polymers, flame retardants, and inorganic materials. Compared to pure water and 3.5 wt% MgCl2 solution, the as-prepared hydrogel presents good fire prevention performance. In addition, it is found that CO and CO2 are not produced by coal when the pyrolysis temperature is lower than 200°C. During low-temperature pyrolysis, CO is more likely to be produced than CO2, indicating inadequate pyrolysis behavior. At the same time, the addition of fire-preventing hydrogel can not only decrease the maximum CO2 concentration before… More > Graphic Abstract

    Effect of Bio-Based Organic‒Inorganic Hybrid Hydrogels on Fire Prevention of Spontaneous Combustion of Coals

  • Open Access

    PROCEEDINGS

    Hydrogels with Brain Tissue-Like Mechanical Properties in Complex Environments

    Jingyu Wang1,#, Yongrou Zhang4,#, Zuyue Lei1, Junqi Wang1, Yangming Zhao1, Taolin Sun3,*, Zhenyu Jiang1, Licheng Zhou1, Zejia Liu1, Yiping Liu1, Bao Yang1, Liqun Tang1,2,*

    The International Conference on Computational & Experimental Engineering and Sciences, Vol.25, No.4, pp. 1-1, 2023, DOI:10.32604/icces.2022.08829

    Abstract In surgical training applications and experimental research, brain tissues immersed in cerebrospinal fluid often involve very complex deformation and strain rate effects, which affects their reliability and stability. Thus, it is indispensable to develop a high-fidelity human brain tissue simulant material as a physical surrogate model to understand their mechanical behavior, such as traumatic brain injury (TBI). However, the reported simulant materials have not yet been able to compare and satisfy the above two mechanical properties. Here, we developed a novel composite hydrogel with brain tissue-like mechanical properties and investigated their mechanical behavior in a… More >

  • Open Access

    PROCEEDINGS

    Experimental Investigation on Pure-Shear Ratcheting Behavior of Double-Network Tough Hydrogels

    Xuelian Zhang1, Junjie Liu1,*, Jian Li2, Zhihong Liang1, Han Jiang1, Guozheng Kang1, Qianhua Kan1,*

    The International Conference on Computational & Experimental Engineering and Sciences, Vol.25, No.3, pp. 1-1, 2023, DOI:10.32604/icces.2023.010142

    Abstract The last decades have witnessed the real and huge potential applications of hydrogels in various areas, including biomedicine, soft robotics, and flexible electronics. The fatigue of hydrogels challenges their reliability and longevity in service, but the related works are not sufficient. In this work, stress-controlled cyclic fatigue tests of a double-network tough hydrogel, consisting of polyacrylamide and alginate polymer networks, under pure shear deformation are investigated. The effects of peak stress, loading rate, peak stress holding time, and environmental relative humidity on the fatigue of the double-network tough hydrogel are considered. The results show that… More >

  • Open Access

    ARTICLE

    Fabricating Cationic Lignin Hydrogels for Dye Adsorption

    Chao Wang, Xuezhen Feng, Wanbing Li, Shibin Shang*, Haibo Zhang*

    Journal of Renewable Materials, Vol.11, No.4, pp. 1793-1805, 2023, DOI:10.32604/jrm.2023.024521 - 01 December 2022

    Abstract Due to the low content of adsorption-active groups in lignin, its application in the field of adsorption is limited. Herein, we first prepared cationic kraft lignin acrylate, from which a cationic lignin (CKLA) hydrogel was further prepared by cationic kraft lignin acrylate, acrylamide, and N, N’-methylenebisacrylamide. The morphology, compression properties and swelling properties of CKLA hydrogels were investigated. The prepared CKLA hydrogel was applied as an adsorbent for Congo red. The effect of CKLA hydrogel dosages, initial concentration of Congo red, and pH on adsorption efficiency was investigated. The maximum Congo red removal efficiency was More >

  • Open Access

    ARTICLE

    Nano-CaO2 Promotes the Release of Carbon Sources from Municipal Sludge and the Preparation of Double-Network Hydrogels with High Swelling Ratios

    Yalin Li1,2,*, Yu Huang2, Lei Liu1, Haozhao Liu1, Haiyang He1, Dongxue Lu1, Tingting Dong1

    Journal of Renewable Materials, Vol.11, No.3, pp. 1237-1253, 2023, DOI:10.32604/jrm.2022.022972 - 31 October 2022

    Abstract

    In this study, hydrogels were prepared from municipal sludge to recycle and realize the value-added utilization of the carbon components in this abundant waste material. The carbon sources were extracted from the municipal sludge using synthesised nano CaO2 as an oxidant, and the carbon sources were graft copolymerised with acrylic acid monomer using N, N′-methylenebisacrylamide as a crosslinking agent and ammonium persulfate as an initiator. The factors influencing the hydrogel preparation were investigated by single-factor experiments. Based on the results of the single-factor experiments, a hydrogel with a swelling ratio of up to 19768.4% at 12

    More > Graphic Abstract

    Nano-CaO<sub>2</sub> Promotes the Release of Carbon Sources from Municipal Sludge and the Preparation of Double-Network Hydrogels with High Swelling Ratios

  • Open Access

    ARTICLE

    Synthesis and Properties of Rosin-Based Composite Acrylamide Hydrogels

    Shuangsheng Zhang, Bin Sun, Siyu Li, Xiangyu Lin, Muhua Chen*, Xu Xu*

    Journal of Renewable Materials, Vol.11, No.2, pp. 853-865, 2023, DOI:10.32604/jrm.2022.022901 - 22 September 2022

    Abstract Hydrogels have been widely applied in agricultural drought-resistance, pollution regulation, drug delivery and so on. Acrylamide (AM) is usually used as raw material to synthesize acrylamide hydrogels. However, inherently low mechanical strength greatly limits their applications in some special areas. Therefore, it is necessary to choose suitable functional monomers to optimize acrylamide hydrogels and improve their mechanical performances. In this paper, a novel acrylamide monomer modified by rosin was synthesized, and then polyacrylamide/rosin-based acrylamide (RAM) composite hydrogels were prepared via free radical polymerization using potassium persulfate as initiator, N, N′-methylene-bisacrylamide (MBA) as a crosslinker. The… More > Graphic Abstract

    Synthesis and Properties of Rosin-Based Composite Acrylamide Hydrogels

  • Open Access

    ARTICLE

    Synthesis and Characterization of Hydrogels Based on Potato Starch/Poly(vinyl Alcohol)/N,N′-Methylenebisacrylamide

    Diego David Pinzón-Moreno*, Eder Clidio Vicuña-Galindo, José Vulfrano González-Fernández, José Luis Soto-Gonzales, María Verónica Carranza-Oropeza*

    Journal of Renewable Materials, Vol.10, No.8, pp. 2179-2201, 2022, DOI:10.32604/jrm.2022.019793 - 25 April 2022

    Abstract Several hydrogels were synthesized by free-radical polymerization in an aqueous medium based on potato starch (PS), poly(vinyl alcohol) (PVA), and N,N′-Methylenebisacrylamide (MBAm), being possible to study these hydrogels as a function of the proportion of components incorporated. In this way, the products generated from the synthesis were characterized by swelling and deswelling kinetics, the first swelling being verified with Schott and statistical models, allowing to contrast the proximity between the experimental and theoretical behavior. Additionally, water retention in soil (R%), spectroscopy (FTIR), morphological (SEM), and thermal (TGA and DSC) analysis allowing to know the intrinsic More >

  • Open Access

    VIEWPOINT

    Mesenchymal stem cells, secretome and biomaterials in in-vivo animal models: Regenerative medicine application in cutaneous wound healing

    MASSIMO CONESE1,*, AURELIO PORTINCASA2

    BIOCELL, Vol.46, No.8, pp. 1815-1826, 2022, DOI:10.32604/biocell.2022.019448 - 22 April 2022

    Abstract The treatment of nonhealing and chronic cutaneous wounds still needs a clinical advancement to be effective. Both mesenchymal stem cells (MSCs), obtained from different sources, and their secretome derived thereof (especially exosomes) can activate signaling pathways related to promotion of cell migration, vascularization, collagen deposition, and inflammatory response demonstrating prohealing, angiogenetic and anti-scarring capacities. On the other hand, biodegradable biomimetic scaffolds can facilitate endogenous cell attachment and proliferation as well as extracellular matrix production. In this Review, we revise the complex composites made by biomimetic scaffolds, mainly hydrogels, and MSC-derived exosomes constructed for cutaneous wound More >

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