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    Three-Dimensional Discrete Element Simulation of Electrode Structural Evolutions in Lithium-Ion Batteries During Drying and Calendering

    Yuhang Lyu1, Shaohai Dong1, Li Ting Gao1, Zhan-Sheng Guo1,*

    The International Conference on Computational & Experimental Engineering and Sciences, Vol.30, No.3, pp. 1-1, 2024, DOI:10.32604/icces.2024.012815

    Abstract Drying and calendering processes are crucial in electrode manufacturing, as they significantly affect the mechanical and electrochemical performances of lithium-ion batteries. In this study, we established a three-dimensional (3D) representative volume element (RVE) of electrodes composed of active material particles, carbon binder domain particles, solvent, and different particle contact types. We continuously simulated the 3D macroscopic and microscopic structural evolutions of the RVE during drying and calendering using the discrete element method (DEM). Based on the evolution of the particle coordination numbers and contact networks during drying, we propose a three-stage-drying scheme, consistent with the More >

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