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  • Open Access

    ARTICLE

    Eco-Friendly Particleboards Produced with Banana Tree (Musa paradisiaca) Pseudostem Fibers Bonded with Cassava Starch and Urea-Formaldehyde Adhesives

    Prosper Mensah1, Rafael Rodolfo de Melo2, Edgley Alves de Oliveira Paula2, Alexandre Santos Pimenta3, Juliana de Moura2, Fernando Rusch2,*

    Journal of Renewable Materials, Vol.13, No.7, pp. 1475-1489, 2025, DOI:10.32604/jrm.2025.02025-0047 - 22 July 2025

    Abstract The increase in wood and wood-based products in the construction and furniture sectors has grown exponentially, generating severe environmental and socioeconomic impacts. Particleboard panels have been the main cost-benefit option on the market due to their lightness and lower cost compared to solid wood. However, the synthetic adhesives used in producing traditional particleboard panels cause serious harm to human health. Developing particleboard panels with fibrous waste and natural adhesives could be a sustainable alternative for these sectors. The work aimed to create particleboards with fibrous wastes from the pseudostem of the banana tree (Musa paradisiaca) and… More > Graphic Abstract

    Eco-Friendly Particleboards Produced with Banana Tree (<i>Musa paradisiaca</i>) Pseudostem Fibers Bonded with Cassava Starch and Urea-Formaldehyde Adhesives

  • Open Access

    ARTICLE

    Facile Crosslinking of Hardwood Kraft Lignin for Sustainable Bio-Based Wood Adhesives

    Ega Cyntia Watumlawar1, Byung-Dae Park1,*, Long Yang2, Guanben Du2

    Journal of Renewable Materials, Vol.13, No.5, pp. 829-848, 2025, DOI:10.32604/jrm.2025.02024-0056 - 20 May 2025

    Abstract As the most abundant aromatic bio-based polymer, lignin has great potential as a sustainable feedstock for building crosslinked thermoset polymers as bio-based adhesives. However, the potential of hardwood kraft lignin (HKL) is limited due to its poor crosslinking reactivity. Hence, for the first time, the present study reports the facile oxidation of HKL involving a redox reaction with silver-ammonia complexes ([(AgNH3)2]+), primarily focusing on oxidation to produce reactive quinones and promote C–C linkages during reaction. This study aims to increases reactivity of oxidized HKL for effective crosslinking with monoethanolamine (MEA) for the development of bio-based wood… More > Graphic Abstract

    Facile Crosslinking of Hardwood Kraft Lignin for Sustainable Bio-Based Wood Adhesives

  • Open Access

    REVIEW

    Nanocellulose-Based Adhesives for Sustainable Wood-Polymer Composites: Recent Advancement and Future Perspective

    Amelia Hariry1, Efri Mardawati1,2,*, Apri Heri Iswanto3, Tati Karliati4, Lukmanul Hakim Zaini5,6,*, Muhammad Adly Rahandi Lubis2,7

    Journal of Renewable Materials, Vol.13, No.4, pp. 773-798, 2025, DOI:10.32604/jrm.2025.058359 - 21 April 2025

    Abstract Nanocellulose-based adhesives are gaining attention as a viable alternative to conventional adhesives, offering benefits such as cost-effectiveness and scalability, which make them suitable for various sectors, including cosmetics, pharmaceuticals, biodegradable products, and as reinforcing agents in natural adhesives. This review delves into the current advancements in nanocellulose-based adhesive solutions for sustainable and eco-friendly wood composites, using systematic review methods and bibliometric analysis. Data were collected from the Scopus database, spanning from 2007 to 2024, and visualized using VOSviewer to highlight emerging trends in the field. The analysis revealed that nanocellulose shows great potential as a More >

  • Open Access

    ARTICLE

    Preparation of Flaxseed Meal Protein Renewable Bioadhesive by Using Small Proportions of Trimethylolpropane Trigglycidyl Ether and Ethylenediamine

    Chenglong Zhong1, Xianfeng Hou1,*, Shuai Peng1, Zhenzhong Gao1, Qiaofang Zhou1, Shijing Yan2

    Journal of Renewable Materials, Vol.13, No.2, pp. 297-310, 2025, DOI:10.32604/jrm.2024.049534 - 20 February 2025

    Abstract The main raw material utilized in wood adhesives comes from petrochemical extractives. However, due to the excessive dependence on petrochemical resources and the adverse impact on the ecosystem and human well-being, there is an increasing trend to develop byproduct protein-based adhesives in the current global food safety context. In this research, flaxseed meal was subjected to pretreatment, and trimethylolpropane triglycidyl ether (TTE) and ethylenediamine (EN) were utilized as crosslinkers to establish a more compact adhesive layer and to prevent water intrusion. The pretreatment decreased the FM/UB viscosity by 60% compared to FM. The combination… More > Graphic Abstract

    Preparation of Flaxseed Meal Protein Renewable Bioadhesive by Using Small Proportions of Trimethylolpropane Trigglycidyl Ether and Ethylenediamine

  • Open Access

    REVIEW

    Recent Developments in Bioadhesives and Binders

    Hong Lei1, Xiaojian Zhou2, Antonio Pizzi3,*, Guanben Du2,*, Xuedong Xi2

    Journal of Renewable Materials, Vol.13, No.2, pp. 199-249, 2025, DOI:10.32604/jrm.2025.02024-0048 - 20 February 2025

    Abstract This review is composed of three main parts each of which is written by well-known top specialists that have been, in a way or other, also the main participants of the majority of the developments reported. Thus, after a general part covering the grand lines and more in-depth views of more recent tannin, lignin, carbohydrate and soy bioadhesives, some mix of the other bio raw materials with soy protein and soy flour and some other differently sourced bioadhesives for wood, this review presents a more in-depth part on starch-based wood adhesives and a more in-depth… More > Graphic Abstract

    Recent Developments in Bioadhesives and Binders

  • Open Access

    REVIEW

    Overview of the Synthesis, Characterization, and Application of Tannin-Glyoxal Adhesive for Wood-Based Composites

    Awanda Wira Anggini1,2, Rita Kartika Sari2, Efri Mardawati3,4, Tati Karliati5, Apri Heri Iswanto6, Muhammad Adly Rahandi Lubis1,4,*

    Journal of Renewable Materials, Vol.12, No.7, pp. 1165-1186, 2024, DOI:10.32604/jrm.2024.051854 - 21 August 2024

    Abstract More than a century after its initial synthesis, urea-formaldehyde (UF) resins still have dominant applications as adhesives, paints, and coatings. However, formaldehyde in this industry produces formaldehyde emissions that are dangerous to health. Scientists have spent the last decade replacing formaldehyde and phenol with environmentally friendly substances such as glyoxal and tannin to create bio-based adhesives. This review covers recent advances in synthesizing glyoxal tannin-based resins, especially those made from sustainable raw material substitutes and changes made to synthetic processes to improve mechanical properties. The efficacy of using tannin-glyoxal adhesives in producing wood-based composites has… More > Graphic Abstract

    Overview of the Synthesis, Characterization, and Application of Tannin-Glyoxal Adhesive for Wood-Based Composites

  • Open Access

    ARTICLE

    Structural Elucidation of the Polymeric Condensed Tannins of Acacia nilotica Subspecies by 13C NMR, MALDI-TOF and TMA as Sources of Bioadhesives

    Zeinab Osman1,2,3,*, Antonio Pizzi2,*, Bertrand Charrier3

    Journal of Renewable Materials, Vol.12, No.7, pp. 1291-1310, 2024, DOI:10.32604/jrm.2024.051619 - 21 August 2024

    Abstract Tannin was extracted from different subspecies of Acacia nilotica, Acacia nilotica nilotica (Ann), Acacia nilotica tomentosa (Ant) and Acacia nilotica adansonii (Ana). The aim was to elucidate their structure and evaluate their reactivity as bioadhesives in the wood industry. The extracts were prepared by hot water extraction (90°C temperature). Their gel time with paraformaldehyde was used at first to compare their reactivity. The tannin contents and the percentage of total polyphenolic materials in different solutions of the extracts spray dried powder were determined by the hide powder method. Concentrated solutions (47%) were tested by both MALDI ToF, CNMR.… More > Graphic Abstract

    Structural Elucidation of the Polymeric Condensed Tannins of <i>Acacia nilotica</i> Subspecies by <sup>13</sup>C NMR, MALDI-TOF and TMA as Sources of Bioadhesives

  • Open Access

    ARTICLE

    Adhesion of Technical Lignin-Based Non-Isocyanate Polyurethane Adhesives for Wood Bonding

    Jaewook Lee1, Byung-Dae Park1,*, Qinglin Wu2

    Journal of Renewable Materials, Vol.12, No.7, pp. 1187-1205, 2024, DOI:10.32604/jrm.2024.049948 - 21 August 2024

    Abstract Lignin is the most abundant aromatic natural polymer, and receiving great attention in replacing various petroleum-based polymers. The aim of this study is to investigate the feasibility of technical lignin as a polyol for the synthesis of non-isocyanate polyurethane (NIPU) adhesives to substitute current polyurethane (PU) adhesives that have been synthesized with toxic isocyanate and polyols. Crude hardwood kraft lignin (C-HKL) was extracted from black liquor from a pulp mill followed by acetone fractionation to obtain acetone soluble-HKL (AS-HKL). Then, C-HKL, AS-HKL, and softwood sodium lignosulfonate (LS) were used for the synthesis of technical lignin-based… More > Graphic Abstract

    Adhesion of Technical Lignin-Based Non-Isocyanate Polyurethane Adhesives for Wood Bonding

  • Open Access

    ARTICLE

    Properties of Bark Particleboard Bonded with Demethylated Lignin Adhesives Derived from Leucaena leucocephala Bark

    Rafidah Md Salim1,2,*, Jahimin Asik2, Mohd Sani Sarjadi2

    Journal of Renewable Materials, Vol.12, No.4, pp. 737-769, 2024, DOI:10.32604/jrm.2024.045695 - 12 June 2024

    Abstract Lignin extraction from bark can maximize the utilization of biomass waste, offer cost-effectiveness, and promote environmental friendliness when employed as an adhesive material in bark particleboard production. Particles of fine (0.2 to 1.0 mm), medium (1.0 to 2.5 mm), and coarse (2.5 to 12.0 mm) sizes, derived from the bark of Leucaena leucocephala, were hot-pressed using a heating plate at 175°C for 7 min to create single-layer particleboards measuring 320 mm × 320 mm × 10 mm, targeting a density of 700 kg/m. Subsequently, the samples were trimmed and conditioned at 20°C and 65% relative humidity.… More > Graphic Abstract

    Properties of Bark Particleboard Bonded with Demethylated Lignin Adhesives Derived from <i>Leucaena leucocephala</i> Bark

  • Open Access

    ARTICLE

    Preparation of Environmentally Friendly Urea-Hexanediamine-Glyoxal (HUG) Resin Wood Adhesive

    Qianyu Zhang1,2,#, Shi Chen1,2,#, Long Cao1,2, Hong Lei3, Antonio Pizzi4, Xuedong Xi1,2,*, Guanben Du1,2

    Journal of Renewable Materials, Vol.12, No.2, pp. 235-244, 2024, DOI:10.32604/jrm.2023.029537 - 11 March 2024

    Abstract Using non-toxic, low-volatile glyoxal to completely replace formaldehyde for preparing urea-glyoxal (UG) resin adhesive is a hot research topic that could be of great interest for the wood industry. However, urea-glyoxal (UG) resins prepared by just using glyoxal instead of formaldehyde usually yields a lower degree of polymerization. This results in a poorer bonding performance and water resistance of UG resins. A good solution is to pre-react urea to preform polyurea molecules presenting already a certain degree of polymerization, and then to condense these with glyoxal to obtain a novel UG resin. Therefore, in this… More > Graphic Abstract

    Preparation of Environmentally Friendly Urea-Hexanediamine-Glyoxal (HUG) Resin Wood Adhesive

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