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  • Open Access

    ARTICLE

    Sustainable Particleboards Based on Sugarcane Bagasse and Bonded with a Waste-Grown Black Soldier Fly Larvae Commercial Flour-Based Adhesive: Rheological, Physical, and Mechanical Properties

    Francisco Daniel García1,2, Solange Nicole Aigner1,2, Natalia Raffaeli3, Antonio José Barotto3, Eleana Spavento3, Mariano Martín Escobar1,4, Marcela Angela Mansilla1,4, Alejandro Bacigalupe1,4,*

    Journal of Renewable Materials, Vol.14, No.1, 2026, DOI:10.32604/jrm.2025.02025-0181 - 23 January 2026

    Abstract This study explores the use of black soldier fly larvae protein as a bio-based adhesive to produce particleboards from sugarcane bagasse. A comprehensive evaluation was conducted, including rheological characterization of the adhesive and physical–mechanical testing of the panels according to European standards. The black soldier fly larvae-based adhesive exhibited gel-like viscoelastic behavior, rapid partial structural recovery after shear, and favorable application properties. Particleboards manufactured with this adhesive and sugarcane bagasse achieved promising mechanical performance, with modulus of rupture and modulus of elasticity values of 30.2 and 3500 MPa, respectively. Internal bond strength exceeded 0.4 MPa,… More > Graphic Abstract

    Sustainable Particleboards Based on Sugarcane Bagasse and Bonded with a Waste-Grown Black Soldier Fly Larvae Commercial Flour-Based Adhesive: Rheological, Physical, and Mechanical Properties

  • Open Access

    ARTICLE

    Plywood Bio-Adhesives by Oxidized Lignin Urea Bridged with Oxidized Starch

    Hamed Younesi-Kordkheili1,*, Antonio Pizzi2,*

    Journal of Renewable Materials, Vol.14, No.1, 2026, DOI:10.32604/jrm.2025.02025-0179 - 23 January 2026

    Abstract The aim of this research was to synthesize a new totally bio wood adhesive entailing the use of oxidized starch (OST), urea, and oxidized lignin (OL). For this reason, non-modified (L) and oxidized lignin (OL) at different contents (20%, 30%, and 40%) were used to prepare the starch-urea-lignin (SUL) and starch-urea-oxidized lignin (SUOL) resin. Sodium persulfate (SPS) as oxidizer was employed to oxidize both starch and lignin. Urea was just used as a low cost and effective crosslinker in the resin composition. The properties of the synthesized resins and the plywood panels bonded with them… More > Graphic Abstract

    Plywood Bio-Adhesives by Oxidized Lignin Urea Bridged with Oxidized Starch

  • Open Access

    ARTICLE

    Eco-Friendly Particleboards Produced with Banana Tree (Musa paradisiaca) Pseudostem Fibers Bonded with Cassava Starch and Urea-Formaldehyde Adhesives

    Prosper Mensah1, Rafael Rodolfo de Melo2, Edgley Alves de Oliveira Paula2, Alexandre Santos Pimenta3, Juliana de Moura2, Fernando Rusch2,*

    Journal of Renewable Materials, Vol.13, No.7, pp. 1475-1489, 2025, DOI:10.32604/jrm.2025.02025-0047 - 22 July 2025

    Abstract The increase in wood and wood-based products in the construction and furniture sectors has grown exponentially, generating severe environmental and socioeconomic impacts. Particleboard panels have been the main cost-benefit option on the market due to their lightness and lower cost compared to solid wood. However, the synthetic adhesives used in producing traditional particleboard panels cause serious harm to human health. Developing particleboard panels with fibrous waste and natural adhesives could be a sustainable alternative for these sectors. The work aimed to create particleboards with fibrous wastes from the pseudostem of the banana tree (Musa paradisiaca) and… More > Graphic Abstract

    Eco-Friendly Particleboards Produced with Banana Tree (<i>Musa paradisiaca</i>) Pseudostem Fibers Bonded with Cassava Starch and Urea-Formaldehyde Adhesives

  • Open Access

    ARTICLE

    Facile Crosslinking of Hardwood Kraft Lignin for Sustainable Bio-Based Wood Adhesives

    Ega Cyntia Watumlawar1, Byung-Dae Park1,*, Long Yang2, Guanben Du2

    Journal of Renewable Materials, Vol.13, No.5, pp. 829-848, 2025, DOI:10.32604/jrm.2025.02024-0056 - 20 May 2025

    Abstract As the most abundant aromatic bio-based polymer, lignin has great potential as a sustainable feedstock for building crosslinked thermoset polymers as bio-based adhesives. However, the potential of hardwood kraft lignin (HKL) is limited due to its poor crosslinking reactivity. Hence, for the first time, the present study reports the facile oxidation of HKL involving a redox reaction with silver-ammonia complexes ([(AgNH3)2]+), primarily focusing on oxidation to produce reactive quinones and promote C–C linkages during reaction. This study aims to increases reactivity of oxidized HKL for effective crosslinking with monoethanolamine (MEA) for the development of bio-based wood… More > Graphic Abstract

    Facile Crosslinking of Hardwood Kraft Lignin for Sustainable Bio-Based Wood Adhesives

  • Open Access

    REVIEW

    Nanocellulose-Based Adhesives for Sustainable Wood-Polymer Composites: Recent Advancement and Future Perspective

    Amelia Hariry1, Efri Mardawati1,2,*, Apri Heri Iswanto3, Tati Karliati4, Lukmanul Hakim Zaini5,6,*, Muhammad Adly Rahandi Lubis2,7

    Journal of Renewable Materials, Vol.13, No.4, pp. 773-798, 2025, DOI:10.32604/jrm.2025.058359 - 21 April 2025

    Abstract Nanocellulose-based adhesives are gaining attention as a viable alternative to conventional adhesives, offering benefits such as cost-effectiveness and scalability, which make them suitable for various sectors, including cosmetics, pharmaceuticals, biodegradable products, and as reinforcing agents in natural adhesives. This review delves into the current advancements in nanocellulose-based adhesive solutions for sustainable and eco-friendly wood composites, using systematic review methods and bibliometric analysis. Data were collected from the Scopus database, spanning from 2007 to 2024, and visualized using VOSviewer to highlight emerging trends in the field. The analysis revealed that nanocellulose shows great potential as a More >

  • Open Access

    ARTICLE

    Preparation of Flaxseed Meal Protein Renewable Bioadhesive by Using Small Proportions of Trimethylolpropane Trigglycidyl Ether and Ethylenediamine

    Chenglong Zhong1, Xianfeng Hou1,*, Shuai Peng1, Zhenzhong Gao1, Qiaofang Zhou1, Shijing Yan2

    Journal of Renewable Materials, Vol.13, No.2, pp. 297-310, 2025, DOI:10.32604/jrm.2024.049534 - 20 February 2025

    Abstract The main raw material utilized in wood adhesives comes from petrochemical extractives. However, due to the excessive dependence on petrochemical resources and the adverse impact on the ecosystem and human well-being, there is an increasing trend to develop byproduct protein-based adhesives in the current global food safety context. In this research, flaxseed meal was subjected to pretreatment, and trimethylolpropane triglycidyl ether (TTE) and ethylenediamine (EN) were utilized as crosslinkers to establish a more compact adhesive layer and to prevent water intrusion. The pretreatment decreased the FM/UB viscosity by 60% compared to FM. The combination… More > Graphic Abstract

    Preparation of Flaxseed Meal Protein Renewable Bioadhesive by Using Small Proportions of Trimethylolpropane Trigglycidyl Ether and Ethylenediamine

  • Open Access

    REVIEW

    Recent Developments in Bioadhesives and Binders

    Hong Lei1, Xiaojian Zhou2, Antonio Pizzi3,*, Guanben Du2,*, Xuedong Xi2

    Journal of Renewable Materials, Vol.13, No.2, pp. 199-249, 2025, DOI:10.32604/jrm.2025.02024-0048 - 20 February 2025

    Abstract This review is composed of three main parts each of which is written by well-known top specialists that have been, in a way or other, also the main participants of the majority of the developments reported. Thus, after a general part covering the grand lines and more in-depth views of more recent tannin, lignin, carbohydrate and soy bioadhesives, some mix of the other bio raw materials with soy protein and soy flour and some other differently sourced bioadhesives for wood, this review presents a more in-depth part on starch-based wood adhesives and a more in-depth… More > Graphic Abstract

    Recent Developments in Bioadhesives and Binders

  • Open Access

    REVIEW

    Overview of the Synthesis, Characterization, and Application of Tannin-Glyoxal Adhesive for Wood-Based Composites

    Awanda Wira Anggini1,2, Rita Kartika Sari2, Efri Mardawati3,4, Tati Karliati5, Apri Heri Iswanto6, Muhammad Adly Rahandi Lubis1,4,*

    Journal of Renewable Materials, Vol.12, No.7, pp. 1165-1186, 2024, DOI:10.32604/jrm.2024.051854 - 21 August 2024

    Abstract More than a century after its initial synthesis, urea-formaldehyde (UF) resins still have dominant applications as adhesives, paints, and coatings. However, formaldehyde in this industry produces formaldehyde emissions that are dangerous to health. Scientists have spent the last decade replacing formaldehyde and phenol with environmentally friendly substances such as glyoxal and tannin to create bio-based adhesives. This review covers recent advances in synthesizing glyoxal tannin-based resins, especially those made from sustainable raw material substitutes and changes made to synthetic processes to improve mechanical properties. The efficacy of using tannin-glyoxal adhesives in producing wood-based composites has… More > Graphic Abstract

    Overview of the Synthesis, Characterization, and Application of Tannin-Glyoxal Adhesive for Wood-Based Composites

  • Open Access

    ARTICLE

    Structural Elucidation of the Polymeric Condensed Tannins of Acacia nilotica Subspecies by 13C NMR, MALDI-TOF and TMA as Sources of Bioadhesives

    Zeinab Osman1,2,3,*, Antonio Pizzi2,*, Bertrand Charrier3

    Journal of Renewable Materials, Vol.12, No.7, pp. 1291-1310, 2024, DOI:10.32604/jrm.2024.051619 - 21 August 2024

    Abstract Tannin was extracted from different subspecies of Acacia nilotica, Acacia nilotica nilotica (Ann), Acacia nilotica tomentosa (Ant) and Acacia nilotica adansonii (Ana). The aim was to elucidate their structure and evaluate their reactivity as bioadhesives in the wood industry. The extracts were prepared by hot water extraction (90°C temperature). Their gel time with paraformaldehyde was used at first to compare their reactivity. The tannin contents and the percentage of total polyphenolic materials in different solutions of the extracts spray dried powder were determined by the hide powder method. Concentrated solutions (47%) were tested by both MALDI ToF, CNMR.… More > Graphic Abstract

    Structural Elucidation of the Polymeric Condensed Tannins of <i>Acacia nilotica</i> Subspecies by <sup>13</sup>C NMR, MALDI-TOF and TMA as Sources of Bioadhesives

  • Open Access

    ARTICLE

    Adhesion of Technical Lignin-Based Non-Isocyanate Polyurethane Adhesives for Wood Bonding

    Jaewook Lee1, Byung-Dae Park1,*, Qinglin Wu2

    Journal of Renewable Materials, Vol.12, No.7, pp. 1187-1205, 2024, DOI:10.32604/jrm.2024.049948 - 21 August 2024

    Abstract Lignin is the most abundant aromatic natural polymer, and receiving great attention in replacing various petroleum-based polymers. The aim of this study is to investigate the feasibility of technical lignin as a polyol for the synthesis of non-isocyanate polyurethane (NIPU) adhesives to substitute current polyurethane (PU) adhesives that have been synthesized with toxic isocyanate and polyols. Crude hardwood kraft lignin (C-HKL) was extracted from black liquor from a pulp mill followed by acetone fractionation to obtain acetone soluble-HKL (AS-HKL). Then, C-HKL, AS-HKL, and softwood sodium lignosulfonate (LS) were used for the synthesis of technical lignin-based… More > Graphic Abstract

    Adhesion of Technical Lignin-Based Non-Isocyanate Polyurethane Adhesives for Wood Bonding

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