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  • Open Access

    SHORT COMMUNICATION

    Preparation of Regenerated Silk Fibroin Hybrid Fibers with Hydrogen Peroxide Sensing Properties by Wet Spinning

    Song Lu1, Jianjun Guo2, Richard Ansah Herman1, Xinyi Wu1, Lin Ma1, Guohua Wu1,*

    Journal of Renewable Materials, Vol.12, No.6, pp. 1043-1055, 2024, DOI:10.32604/jrm.2024.051767 - 02 August 2024

    Abstract Silk is widely used in the production of high-quality textiles. At the same time, the amount of silk textiles no longer in use and discarded is increasing, resulting in significant waste and pollution. This issue is of great concern in many countries where silk is used. Hydrogen peroxide as a naturally occurring compound is an important indicator of detection in both biology and the environment. This study aims to develop a composite fiber with hydrogen peroxide-sensing properties using discarded silk materials. To achieve this goal, firstly, polydopamine (PDA) was used to encapsulate the ZnFeO NPs… More > Graphic Abstract

    Preparation of Regenerated Silk Fibroin Hybrid Fibers with Hydrogen Peroxide Sensing Properties by Wet Spinning

  • Open Access

    ARTICLE

    Rheological Study on Blend Solutions of Non-mulberry Silk Fibroin and Gelatin Biopolymers

    PRITI1,*, RADHA SACHAN2, ROLI PURWAR3

    Journal of Polymer Materials, Vol.40, No.3-4, pp. 205-214, 2023, DOI:10.32381/JPM.2023.40.3-4.6

    Abstract In current research work, we have studied the blending effect of non-mulberry silk fibroin (10% weight/volume basis) and gelatin (20% weight/volume basis) in formic acid. Several blends as SF10G0, SF2G8, SF3G7, SF5G5 and SF0G10 have been made and their rheological behaviour was investigated. The blend solutions were subjected to a steady shear rheological study in the variety of range of shear rates, namely 0.01–500 sec-1 and the viscosities of blend solutions were noticed to decrease in comparison to pure silk solution. The frequency sweep was employed in dynamic rheological tests to determine complex viscosity of More >

  • Open Access

    ARTICLE

    A Novel Method for the Quantitative Detection of Sericin Content in Silk Fiber Based on the Ratio of Aspartate to Alanine

    Yanfei Feng, Jiaming Lin, Longxing Niu, Peng Pan, Xueping Liu, Linling Huang, Ying Guo, Mingzhong Li*

    Journal of Renewable Materials, Vol.11, No.1, pp. 167-184, 2023, DOI:10.32604/jrm.2022.021339 - 10 August 2022

    Abstract The development of a method for the quantitative determination of the sericin content ratio (SCR) is urgently needed for silk refining and the purification of silk fibroin for biomedical applications. In this work, a series of sericin/fibroin mixed samples with known SCRs were prepared by mixing initial samples of extracted sericin and fibroin from Bombyx mori silk. Significant differences were found in the contents of characteristic hydrophilic amino acids abundant in sericin and hydrophobic amino acids abundant in fibroin, and several linear relationships of SCR associated with the content ratios of Ser/Ala, Asp/Ala, Lys/Ala, Asp/Gly and… More > Graphic Abstract

    A Novel Method for the Quantitative Detection of Sericin Content in Silk Fiber Based on the Ratio of Aspartate to Alanine

  • Open Access

    ARTICLE

    Biodegradable and Biocompatible Polyvinyl alcohol/ Silk Fibroin-Based Composite with Improved Strength

    XINGMIN XU1, QINGQING SUN2, AIRONG XU2, XINBAO GUO2

    Journal of Polymer Materials, Vol.39, No.1-2, pp. 167-181, 2022, DOI:10.32381/JPM.2022.39.1-2.11

    Abstract Silk fibroin (SF) with renewability, biocompatibility and biodegradability shows potential application in various fields including biomedicine, tissue engineering, and wearable electronic devices. Herein, SF is used to exert effective reinforcement of polyvinyl alcohol (PVA) composite film to further improve its practicability. As such, PVA/SF composite films were prepared for the first time using a facile approach. The films were characterized to investigate possible interaction of PVA with SF. Meanwhile, systematic investigations have also been completed to explore the influences of PVA/SF mass ratio on the mechanical properties (tensile strength, elongation at break), biodegradability and biocompatibility, More >

  • Open Access

    ARTICLE

    Fabrication of High Toughness Silk Fibroin/Tungsten Disulfide Nanoparticles Hybrid Fiber and Self-Heating Textile by Wet Spinning

    Jianjun Guo1,2, Lingling Jia3, Sandra Senyo Fometu4, Qiang Ma5, Jinjin Wang1, Hang Li1, Lei Jiang5, Guohua Wu1,*

    Journal of Renewable Materials, Vol.10, No.12, pp. 3373-3389, 2022, DOI:10.32604/jrm.2022.021087 - 14 July 2022

    Abstract Traditionally, silkworm silk has been used to make high-quality textiles. Nevertheless, various wastes from silkworm silk textiles that are no longer used are increasing, which is also causing considerable waste and contamination. This issue is causing widespread concern in countries that use more silk. Regenerated silk fibroin (RSF) fibers have been shown to be fragile and tender, which prohibits RSF from being widely used as a structural component. Therefore, enriching the function of silk and enhancing the RSF mechanical properties are important directions to expand the comprehensive utilization of silk products. In the present research,… More >

  • Open Access

    ARTICLE

    Silk Fibroin-Based Hydrogel for Multifunctional Wearable Sensors

    Yiming Zhao1,2, Hongsheng Zhao3, Zhili Wei4, Jie Yuan1, Jie Jian1, Fankai Kong1, Haojiang Xie1, Xingliang Xiong1,2,*

    Journal of Renewable Materials, Vol.10, No.11, pp. 2729-2746, 2022, DOI:10.32604/jrm.2022.019721 - 29 June 2022

    Abstract The flexible wearable sensors with excellent stretchability, high sensitivity and good biocompatibility are signifi- cantly required for continuously physical condition tracking in health management and rehabilitation monitoring. Herein, we present a high-performance wearable sensor. The sensor is prepared with nanocomposite hydrogel by using silk fibroin (SF), polyacrylamide (PAM), polydopamine (PDA) and graphene oxide (GO). It can be used to monitor body motions (including large-scale and small-scale motions) as well as human electrophysiological (ECG) signals with high sensitivity, wide sensing range, and fast response time. Therefore, the proposed sensor is promising in the fields of rehabilitation, More >

  • Open Access

    ARTICLE

    Macromolecule’s Orientation in a Nanofiber by Bubble Electrospinning

    Dan Tian1,*, Danni Yu2, Chunhui He3

    FDMP-Fluid Dynamics & Materials Processing, Vol.17, No.4, pp. 711-720, 2021, DOI:10.32604/fdmp.2021.014290 - 17 May 2021

    Abstract In the search for sustainable alternatives to harmful synthetic fibers, an increasing amount of research focuses on biomimicry and natural fibers. Sea silk is an exceptional textile material. It is a kind of natural silk produced using the long silky filaments secreted by a specific bivalve mollusk (Pinna nobilis); now at edge of extinction. This paper suggests a simple but effective way to prepare artificial sea silk from Mytilus edulis. A sea silk solution is prepared using a Mytilus edulis protein, and a polyvinyl alcohol (PVA) solution is mixed with the sea silk solution in order to produce More >

  • Open Access

    ARTICLE

    A Promising Wound Dressing from Regenerated Silk Fibroin Sponge with Sustain-ed Release of Silver Nanoparticles

    Yang Li#, Xiaoying Zha#, Xingliang Xiong, Yan Zhang, Ying Feng, Haojiang Xie, Linqing Zhang, Qifeng Jiang*

    Journal of Renewable Materials, Vol.9, No.2, pp. 295-310, 2021, DOI:10.32604/jrm.2021.012271 - 15 December 2020

    Abstract A silk fibroin (SF) spongy wound dressing incorporated with silver nanoparticles (Ag-NPs) was developed for biomedical applications. Ag-NPs were efficiently synthesized in situ via ultra violet (UV) with AgNO3 as precursor and silk fibroin as reducing and protecting agent, respectively. After lyophilization, the formed silk fibroin spongy wound dressing (SFWD) exhibited polyporous morphology and inner lamellae structures, with uniform dispersion of Ag-NPs. The porous structure provided SFWD with the ability to absorb tissue exudatealmost 6 times of its own weight, which could guarantee the sustained release of Ag-NPs. By methanol treatment, SFWD showed much improved mechanical properties… More >

  • Open Access

    ARTICLE

    Robust Color Fastness of Dyed Silk Fibroin Film By Coupling Modification Dyeing with Aniline Diazonium Salt

    ZONGQIAN WANG, HAIWEI YANG, JIAN XING, ZHI LIU*

    Journal of Polymer Materials, Vol.36, No.2, pp. 149-159, 2019, DOI:10.32381/JPM.2019.36.02.4

    Abstract Colored silk fibroin (SF) film can change the proportion of transmitted light composition and therefore shows potential application in optoelectronics area. However, few methods are reported for the preparation of colored SF film with good color fastness. Herein, colored SF film was prepared by coupling modification dyeing (CM-dyeing) of SF tyrosine residues in solution. SF film shows excellent color fastness due to the formation of the azo covalent bond formed by electrophilic substitution reaction between SF tyrosine residues and aniline diazonium salt. Furthermore, compared with the undyed film, the dyed SF film is effectively preserved More >

  • Open Access

    ARTICLE

    Selective Adsorption of Ag(I) from Electronic Waste Leachate Using Modified Silk Sericin

    Sijing Zhang1*, Fengjiao Ao1, Yongping Wang2, Junxue Zhao3, Yongliang Ji1, Shuangli Chen1

    Journal of Renewable Materials, Vol.6, No.1, pp. 102-116, 2018, DOI:10.7569/JRM.2017.634154

    Abstract A novel biosorbent was synthesized by grafting bisthiourea (BTU) on a silk sericin (SS) matrix. This biosorbent was denoted as BTU-SS and characterized by Fourier transform infrared spectroscopy (FTIR), zeta potential measurements, elemental analysis, and X-ray photoelectron spectroscopy (XPS). As revealed by the adsorption experiments, both BTU-SS and SS showed low affinity towards coexisting base metallic ions in Ag(I)-Cu(II)-Zn(II)-Ni(II)-Pb(II) electronic waste leachate mixtures, while their adsorption capacities towards Ag(I) reached 30.5 and 10.4 mg·g–1 at a pH of 5.0, respectively. BTU-SS showed higher selectivity towards Ag(I) than SS, as revealed by the Ag(I) partition coefficients More >

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