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  • Open Access

    ARTICLE

    Influence of Formulation and Hot-Pressing Conditions on the Performance of Bio-Based Molasses Adhesive for Plywood

    Jajang Sutiawan1, Alifah Syahfitri2, Sukma Surya Kusumah1, Dede Hermawan2,*, Rita Kartika Sari2, Luthfi Hakim3, Efri Mardawati4,5, Muhammad Adly Rahandi Lubis1,4,*

    Journal of Renewable Materials, Vol.12, No.8, pp. 1383-1397, 2024, DOI:10.32604/jrm.2024.052052 - 06 September 2024

    Abstract Molasses can serve as a natural adhesive for plywood and particleboard. However, several disadvantages remain, including lower dimensional stability and low bonding strength compared to other adhesives. Therefore, modifications are needed to use molasses as an adhesive for plywood. This research aims to improve bio-based molasses (MO) adhesive for plywood using citric acid (CA) adhesive. In addition, this research aims to analyze the effect of adding citric acid and to investigate the optimum hot-pressing temperature to produce the best quality plywood. In the first stage, the molasses and citric acid were combined in a ratio… More > Graphic Abstract

    Influence of Formulation and Hot-Pressing Conditions on the Performance of Bio-Based Molasses Adhesive for Plywood

  • Open Access

    REVIEW

    Overview of the Synthesis, Characterization, and Application of Tannin-Glyoxal Adhesive for Wood-Based Composites

    Awanda Wira Anggini1,2, Rita Kartika Sari2, Efri Mardawati3,4, Tati Karliati5, Apri Heri Iswanto6, Muhammad Adly Rahandi Lubis1,4,*

    Journal of Renewable Materials, Vol.12, No.7, pp. 1165-1186, 2024, DOI:10.32604/jrm.2024.051854 - 21 August 2024

    Abstract More than a century after its initial synthesis, urea-formaldehyde (UF) resins still have dominant applications as adhesives, paints, and coatings. However, formaldehyde in this industry produces formaldehyde emissions that are dangerous to health. Scientists have spent the last decade replacing formaldehyde and phenol with environmentally friendly substances such as glyoxal and tannin to create bio-based adhesives. This review covers recent advances in synthesizing glyoxal tannin-based resins, especially those made from sustainable raw material substitutes and changes made to synthetic processes to improve mechanical properties. The efficacy of using tannin-glyoxal adhesives in producing wood-based composites has… More > Graphic Abstract

    Overview of the Synthesis, Characterization, and Application of Tannin-Glyoxal Adhesive for Wood-Based Composites

  • Open Access

    ARTICLE

    Structural Elucidation of the Polymeric Condensed Tannins of Acacia nilotica Subspecies by 13C NMR, MALDI-TOF and TMA as Sources of Bioadhesives

    Zeinab Osman1,2,3,*, Antonio Pizzi2,*, Bertrand Charrier3

    Journal of Renewable Materials, Vol.12, No.7, pp. 1291-1310, 2024, DOI:10.32604/jrm.2024.051619 - 21 August 2024

    Abstract Tannin was extracted from different subspecies of Acacia nilotica, Acacia nilotica nilotica (Ann), Acacia nilotica tomentosa (Ant) and Acacia nilotica adansonii (Ana). The aim was to elucidate their structure and evaluate their reactivity as bioadhesives in the wood industry. The extracts were prepared by hot water extraction (90°C temperature). Their gel time with paraformaldehyde was used at first to compare their reactivity. The tannin contents and the percentage of total polyphenolic materials in different solutions of the extracts spray dried powder were determined by the hide powder method. Concentrated solutions (47%) were tested by both MALDI ToF, CNMR.… More > Graphic Abstract

    Structural Elucidation of the Polymeric Condensed Tannins of <i>Acacia nilotica</i> Subspecies by <sup>13</sup>C NMR, MALDI-TOF and TMA as Sources of Bioadhesives

  • Open Access

    ARTICLE

    Adhesion of Technical Lignin-Based Non-Isocyanate Polyurethane Adhesives for Wood Bonding

    Jaewook Lee1, Byung-Dae Park1,*, Qinglin Wu2

    Journal of Renewable Materials, Vol.12, No.7, pp. 1187-1205, 2024, DOI:10.32604/jrm.2024.049948 - 21 August 2024

    Abstract Lignin is the most abundant aromatic natural polymer, and receiving great attention in replacing various petroleum-based polymers. The aim of this study is to investigate the feasibility of technical lignin as a polyol for the synthesis of non-isocyanate polyurethane (NIPU) adhesives to substitute current polyurethane (PU) adhesives that have been synthesized with toxic isocyanate and polyols. Crude hardwood kraft lignin (C-HKL) was extracted from black liquor from a pulp mill followed by acetone fractionation to obtain acetone soluble-HKL (AS-HKL). Then, C-HKL, AS-HKL, and softwood sodium lignosulfonate (LS) were used for the synthesis of technical lignin-based… More > Graphic Abstract

    Adhesion of Technical Lignin-Based Non-Isocyanate Polyurethane Adhesives for Wood Bonding

  • Open Access

    ARTICLE

    Properties of Bark Particleboard Bonded with Demethylated Lignin Adhesives Derived from Leucaena leucocephala Bark

    Rafidah Md Salim1,2,*, Jahimin Asik2, Mohd Sani Sarjadi2

    Journal of Renewable Materials, Vol.12, No.4, pp. 737-769, 2024, DOI:10.32604/jrm.2024.045695 - 12 June 2024

    Abstract Lignin extraction from bark can maximize the utilization of biomass waste, offer cost-effectiveness, and promote environmental friendliness when employed as an adhesive material in bark particleboard production. Particles of fine (0.2 to 1.0 mm), medium (1.0 to 2.5 mm), and coarse (2.5 to 12.0 mm) sizes, derived from the bark of Leucaena leucocephala, were hot-pressed using a heating plate at 175°C for 7 min to create single-layer particleboards measuring 320 mm × 320 mm × 10 mm, targeting a density of 700 kg/m. Subsequently, the samples were trimmed and conditioned at 20°C and 65% relative humidity.… More > Graphic Abstract

    Properties of Bark Particleboard Bonded with Demethylated Lignin Adhesives Derived from <i>Leucaena leucocephala</i> Bark

  • Open Access

    ARTICLE

    Effect of Adhesive Type on the Quality of Coconut Shell Charcoal Briquettes Prepared by the Screw Extruder Machine

    Samsudin Anis1,*, Deni Fajar Fitriyana1, Aldias Bahatmaka1, Muhammad Choirul Anwar1, Arsyad Zanadin Ramadhan1, Fajar Chairul Anam1, Raffanel Adi Permana1, Ahmad Jazilussurur Hakim2, Natalino Fonseca Da Silva Guterres3, Mateus De Sousa Da Silva3

    Journal of Renewable Materials, Vol.12, No.2, pp. 381-396, 2024, DOI:10.32604/jrm.2023.047128 - 11 March 2024

    Abstract Indonesia is one of the largest coconut-producing countries in the world. The utilization of coconut shell waste into briquettes will increase the selling value and become a great export opportunity. However, the effect of adhesives on the quality of coconut shell charcoal briquettes made using screw extruder machine has not been widely studied. This study aims to determine the effect of adhesive type on the quality of coconut shell charcoal briquettes. The process of fabricating briquettes in this study included crushing, mixing, blending, pressing, and drying. In the mixing process, 3 types of adhesives were… More > Graphic Abstract

    Effect of Adhesive Type on the Quality of Coconut Shell Charcoal Briquettes Prepared by the Screw Extruder Machine

  • Open Access

    ARTICLE

    Preparation of Environmentally Friendly Urea-Hexanediamine-Glyoxal (HUG) Resin Wood Adhesive

    Qianyu Zhang1,2,#, Shi Chen1,2,#, Long Cao1,2, Hong Lei3, Antonio Pizzi4, Xuedong Xi1,2,*, Guanben Du1,2

    Journal of Renewable Materials, Vol.12, No.2, pp. 235-244, 2024, DOI:10.32604/jrm.2023.029537 - 11 March 2024

    Abstract Using non-toxic, low-volatile glyoxal to completely replace formaldehyde for preparing urea-glyoxal (UG) resin adhesive is a hot research topic that could be of great interest for the wood industry. However, urea-glyoxal (UG) resins prepared by just using glyoxal instead of formaldehyde usually yields a lower degree of polymerization. This results in a poorer bonding performance and water resistance of UG resins. A good solution is to pre-react urea to preform polyurea molecules presenting already a certain degree of polymerization, and then to condense these with glyoxal to obtain a novel UG resin. Therefore, in this… More > Graphic Abstract

    Preparation of Environmentally Friendly Urea-Hexanediamine-Glyoxal (HUG) Resin Wood Adhesive

  • Open Access

    PROCEEDINGS

    Rate Effect of Adhesive Wear Due to Asperity Plowing

    Jianqiao Hu1,2,*, Hengxu Song1, Xiaoming Liu1,2

    The International Conference on Computational & Experimental Engineering and Sciences, Vol.26, No.1, pp. 1-1, 2023, DOI:10.32604/icces.2023.010554

    Abstract Material wear between contact surfaces with relatively sliding can be related to the failure of elevated asperities at small scales. The asperity wear depends on various factors, including material properties, interfacial adhesion, and friction velocity. In this study, using a series of materials characterized by the modified coarse-grained potentials, we studied the rate effect of adhesive wear at the asperity level over a wide range of plowing conditions. The results showed that increasing plowing velocity leads to the transition of the wear mechanism from plasticity-induced asperity smoothing to the formation of fractured debris and thus… More >

  • Open Access

    PROCEEDINGS

    Rate Effect of Adhesive Wear due to Asperity Plowing

    Jianqiao Hu1,2,*, Hengxu Song1, Xiaoming Liu1,2

    The International Conference on Computational & Experimental Engineering and Sciences, Vol.25, No.3, pp. 1-1, 2023, DOI:10.32604/icces.2023.010554

    Abstract Material wear between contact surfaces with relatively sliding can be related to the failure of elevated asperities at small scales. The asperity wear depends on various factors, including material properties, interfacial adhesion, and friction velocity. In this study, using a series of materials characterized by the modified coarse-grained potentials, we studied the rate effect of adhesive wear at the asperity level over a wide range of plowing conditions. The results showed that increasing plowing velocity leads to the transition of the wear mechanism from plasticity-induced asperity smoothing to the formation of fractured debris and thus… More >

  • Open Access

    REVIEW

    Little Secrets for the Successful Industrial Use of Tannin Adhesives: A Review

    Antonio Pizzi*

    Journal of Renewable Materials, Vol.11, No.9, pp. 3403-3415, 2023, DOI:10.32604/jrm.2023.030930 - 20 July 2023

    Abstract This brief article reviews a very particular and quite narrow field, namely what has been done and what is needed to know for tannin adhesives for wood panels to succeed industrially. The present fashionable focus on bioadhesives has led to producing chemical adhesive formulations and approaches for tannin adhesives as a subject of academic publications. These, as good and original they might be, are and will still remain a rather empty academic exercise if not put to the test of real industrial trials and industrial use. They will remain so without the “little” secrets and… More >

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