Retrieval and Regional Distribution Analysis of Ammonia, Sulfur Dioxide and Nitrogen Dioxide in the Urban Environment Using Ultraviolet DOAS Algorithm
Hao Chen1, Jie Xu1, Yibo Hu1, Fuzhou Niu1,*, Zhiyan Li2, Dan Wang2, Guizhong Fu1, Chuanxin Li3,*
CMES-Computer Modeling in Engineering & Sciences, Vol.134, No.2, pp. 1251-1262, 2023, DOI:10.32604/cmes.2022.022279
- 31 August 2022
(This article belongs to the Special Issue: Advanced Intelligent Decision and Intelligent Control with Applications in Smart City)
Abstract Aiming at the in situ and mobile observation of urban environmental air pollution, a portable instrument using ultraviolet spectrum retrieval algorithm was developed based on the basis of Differential Optical Absorption Spectroscopy (DOAS) and multiple-pass cell technique. Typical trace gas pollutants, NH3, SO2, and NO2, were explored using their optical spectral characteristics in deep ultraviolet wavelength range from 210 to 215 nm. The gas concentration was retrieved by Lambert-Beer's law and nonlinear least square method. With an optimized optical alignment, the detection limits of NH3, SO2, NO2 were estimated to be 2.2, 2.3, and 36.2 ppb, respectively. The More >